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MXene (Ti3C2) Vacancy-Confined Single-Atom Catalyst for Efficient Functionalization of CO2
时间:2019-03-20 15:52:15
分类:JACS
作品信息

期刊

JACS

标题

MXene (Ti3C2) Vacancy-Confined Single-Atom Catalyst for Efficient Functionalization of CO2

作者

Di Zhao, Zheng Chen, Wenjuan Yang, Shoujie Liu,  Xun Zhang, Yi Yu, Weng-Chon Cheong, Lirong Zheng, Fuqiang Ren, Guobing Ying, Xing Cao,  Dingsheng Wang, Qing Peng, Guoxiu Wang, and Chen Chen

摘要

Metal single atoms can be stabilized in Ti-deficient vacancies of ultrathin two-dimensional Ti3–xC2Ty MXene nanosheets via a simultaneous self-reduction–stabilization process at room temperature. The obtained single-atom Pt1/Ti3–xC2Ty catalyst can efficiently functionalize greenhouse gas CO2 to high-value-added chemicals of amines under ambient pressure.

原文链接

https://pubs.acs.org/doi/10.1021/jacs.8b13579

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